In my particular case, I want to bind to the IsReadOnly property of a TextBox to set the Content property of a Button? They are both part of the same StackPanel.
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You need to specify the trigger as part of a style -- the Triggers collection on the Button itself can only contain event triggers. With that in mind, a DataTrigger works fine. However, there is a wrinkle: the value from the Trigger Setter won't overwrite a local Content property. So you have to set the default Content in the Style as well. Here's how it looks:
<Button> <!-- Note no content set directly on button -->
<Button.Style>
<Style TargetType="Button">
<Setter Property="Content" Value="You may write!!!" /> <!-- Here is the 'normal' content -->
<Style.Triggers>
<!-- Here is how we bind to another control's property -->
<DataTrigger Binding="{Binding IsReadOnly, ElementName=textBox}" Value="True">
<Setter Property="Content" Value="NO NO NO" /> <!-- Here is the 'override' content -->
</DataTrigger>
</Style.Triggers>
</Style>
</Button.Style>
</Button>
Have you tried this:
<StackPanel x:Name="LayoutRoot">
<Button Width="75" Content="{Binding IsReadOnly, ElementName=textBox, Mode=Default}" />
<TextBox x:Name="textBox" VerticalAlignment="Top" Text="TextBox" />
</StackPanel>
??