Another approach could be to fake the onclick event like this.
jQuery(document).ready(function () {
jQuery('#<%= txtFirstName.ClientID %>').keypress(function (event) {
if (event.keyCode == 13) {
eval($('#<%=lbHello.ClientID %>').attr('href'));
}
});
});
The downside is that you need to use this for all places you need to make default buttons.